Nonlocal correlations in iron pnictides and chalcogenides

Research output: Contribution to journalJournal articleResearchpeer-review

Documents

  • Shinibali Bhattacharyya
  • Kristofer Bjornson
  • Karim Zantout
  • Daniel Steffensen
  • Laura Fanfarillo
  • Andreas Kreisel
  • Roser Valent
  • Andersen, Brian Møller
  • P. J. Hirschfeld

Deviations of low-energy electronic structurse of iron-based superconductors from density-functional-theory predictions have been parametrized in terms of band- and orbital-dependent mass renormalizations and energy shifts. The former have typically been described in terms of a local self-energy within the framework of dynamical mean field theory, while the latter appears to require nonlocal effects due to interband scattering. By calculating the renormalized band structure in both random phase approximation (RPA) and the two-particle self-consistent approximation (TPSC), we show that correlations in pnictide systems like LaFeAsO and LiFeAs can be described rather well by a nonlocal self-energy. In particular, Fermi pocket shrinkage as seen in experiments occurs due to repulsive interband finite-energy scattering. For the canonical iron chalcogenide system FeSe in its bulk tetragonal phase, the situation is, however, more complex since even including momentum-dependent band renormalizations cannot explain experimental findings. We propose that the nearest-neighbor Coulomb interaction may play an important role in band-structure renormalization in FeSe. We further compare our evaluations of nonlocal quasiparticle scattering lifetime within RPA and TPSC with experimental data for LiFeAs.

Original languageEnglish
Article number035109
JournalPhysical Review B
Volume102
Issue number3
Number of pages12
ISSN2469-9950
DOIs
Publication statusPublished - 6 Jul 2020

ID: 247158601